Abstract: : Despite the desired transition toward sustainable and multimodal mobility, few tools have been developed either to quantify mode use diversity or to assess the effects of transportation system enhancements on multimodal travel behaviors. This paper attempts to fill this gap by proposing a methodology to appraise the causal impact of transport supply improvement on the evolution of multimodality levels between 2013 and 2018 in Montreal (Quebec, Canada). First, the participants of two household travel surveys were clustered into types of people (PeTys) to overcome the cross-sectional nature of the data. This allowed changes in travel behavior per type over a five-year period to be evaluated. A variant of the Dalton index was then applied on a series of aggregated (weighted) intensities of use of several modes to measure multimodality. Various sensitivity analyses were carried out to determine the parameters of this indicator (sensitivity to the least used modes, intensity metric, and mode independency). Finally, a difference-in-differences causal inference approach was explored to model the influence of the improvement of three alternative transport services (transit, bikesharing, and station-based carsharing) on the evolution of modal variability by type of people. The results revealed that, after controlling for different socio-demographic and spatial attributes, increasing transport supply had a significant and positive impact on multimodality. This outcome is therefore good news for the mobility of the future as alternative modes of transport emerge. Mobility as a Service (MaaS) and multimodality (or intermodality) are increasingly fashionable concepts in urban transport research. They are generally presented as essential in the move toward more sustainable mobility, even more now that alternatives to the exclusive use of a private car are emerging. Consequently, many projects focus on the development of technologies (such as mobile applications) to integrate several transportation modes. However, there is a lack of knowledge about multimodal behaviors among travelers, their associated attributes, and motivations. Few tools have been proposed to quantify and explain mode use variability. It, therefore, remains difficult for practitioners to measure the impacts of strategies implemented to promote a more diversified mobility. This paper aims at assessing the influence transport supply may have on the multimodality level of travel behaviors over a five-year period. This required first defining an indicator to summarize the intensities of use of several modes of transport. This indicator was calculated by type of people (aggregated by socio-demographic and spatial attributes) using the last two (2013 and 2018) Montreal household surveys. The evolution by type of people between the two surveys was then cross-analyzed with changes in transport supply. To this end, a difference-in-differences approach that allows causal inference was applied. As a result, this paper provides a means to guide interventions to increase multimodality. This paper is organized as follows. First, some former studies into analyzing and quantifying multimodal mobility, as well as factors affecting multimodal travel behavior, are reviewed. The household surveys used in this paper are then described, and some methodological elements are exposed. The results are reported in three parts: the typology of people is presented; a multimodality indicator is then applied by type; and the causal effect of transport supply on the evolution of multimodality between 2013 and 2018 is modeled. Finally, the paper is concluded and the discussion feeds into the programming of future work.